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The development of efficient unimolecular visible light photoinitiators (PIs) with photobleaching capability, which is essential for various biomedical applications and photopolymerization of thick materials, remains an emerging challenge. Comparisons with reference compounds will also be presented to evidence the interest of coumarins as light absorbing materials for the design of oxime esters. ![]() In this review, an overview of the recent development concerning coumarin-based oxime esters is presented. Face to these considerations, coumarins were thus identified as a promising scaffold for the design of Type I photoinitiators and especially of oxime esters. Using these structures, efficient multicomponent photoinitiating systems could be prepared. In this field, coumarins have been extensively studied as Type II photoinitiators in combination with various additives. 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